You could do it as a desktop app, but what benefit(s) are you looking for?
If you already have it as a WebApp then all that's needed is a web browser (you already have the cross-browser stuff figured out) and by making it a desktop app you'll need to create an installer and keep better track of versioning. Performance wise you probably wont notice much of a change (if at all) because the desktop app will still need to connect to the DB server to get/save the data, which will still take time on a desktop app to do because of the sheer amount of data being passed back.
Really what'll make a difference is the UI control you can use in a desktop app vs a webapp, but that's not what their complaints are.
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Currently using: VS 2005 & 2008 Pro w/sp1 on Win7 Ultimate x64.

There are 3 kinds of people in the world: Those who can count and those who can't.
4 out of 3 people have trouble with fractions.
Windows has a 64 bit GUI for a set of 32 bit extensions on a 16 bit shell for an 8 bit OS using a 4 bit kernel made by a 2 bit company that can't stand 1 bit of competition.
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